For me it would be:
Orikasa Ai
Mastumoto Rica: Outlaw Star/Jim Hawking, Dirty Pair Flash/Kei.
Hayashibara Megumi (well over 100 roles, I use to have a web fan web page for her)
{The above 3 are also really good singers, (I really like Rica Mastumoto), and I have managed to get all of thier solo albums.}
Mitsuishi Kotono : Excel, Misato/NGE, Mink/Drsagon Half, Ebichu, Sailor Moon.
And a few others that I know by voice but not by name.
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